Water Vapor Instrument in the Tropics during Pre AVE and Earlier Aircraft Campaigns Implications for the Seasonal Cycle of Stratospheric Water Vapor and Aura Validation

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Intercomparisons with the Harvard in situ water vapor instrument in the tropics during Pre-AVE and earlier aircraft campaigns: Implications for the seasonal cycle of stratospheric water vapor and Aura validation E. M. Weinstock, J. V. Pittman, D.S. Sayres, J. B. Smith, J. R. Spackman, S. S. Leroy, J. G. Anderson and S. C. Wofsy Harvard University Differences between measurements designed to be close in space and time (Rosenlof, 2003) before flight date HALOE 120 40 CMDL FP 120 tropopause 40 Aircraft/Balloon/Satellite comparison, Pre-AVE, Galapagos, 2004 364 (a) Mixing from northern hemisphere carbon dioxide (ppmv) 362 360 358 356 364 951105 960213 960801 960808 961211 970923 (carbon dioxide boundary condition) (b) Mixing from southern hemisphere (water vapor saturation mixing ratios) carbon dioxide (ppmv) 362 360 358 356 1995 951105 960213 960801 960808 961211 970923 (carbon dioxide boundary condition) 1996 1997 1998 date airmass crossed the 390 K isentrope Constraints on the seasonal cycle of stratospheric water vapor using in situ measurements from the ER-2 and a CO photochemical clock How do we resolve the differences exhibited by water vapor instruments? 1. More intercomparisons followed by organized laboratory intercomparisons and validation with full PI participation. 2. Independent evaluation of instrument performance and accuracy. 3. A national calibration facility under independent oversight. Illustration of the implications of Pre-AVE intercomparison data on the corresponding tropopause temperatures. Calibration source tied to vapor pressure of water at room temperature Source of H2O unperturbed H2O Detection axis Ambient air Laboratory calibration Less than 5% <2 <5 <1 Calibration in flight Uncertainties in water vapor measurement

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