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MATERIALS AND METHODS



Bacterial strains and growth conditions



All bacterial strains and plasmids used in this work are listed in Table S1. The



pneumococcal strains were grown in casein tryptone (CAT) medium containing (per liter)



167 mmol of K2HPO4, 5 mg of choline chloride, 5 g of tryptone, 10 g of enzymatic casein



hydrolysate, 1 g of yeast extract, and 5 g of NaCl (5). After sterilization, glucose was



added to a concentration of 0.2%. S. pneumoniae was grown at 37C, and growth was



monitored by measuring OD at 550 nm or 492 nm. E. coli was grown in Luria-Bertani



(LB) medium (7) at 37C. When appropriate, S. pneumoniae strains were grown in the



presence of 2.5 g ml-1 chloramphenicol, 200 g ml-1 spectinomycin or 2 g ml-1



erythromycin.







Construction of transcriptional fusions and modifications of boxAB2C at the qsrAB



locus



To modify the boxAB2C element at the qsrAB locus, we first amplified a 2700 bp DNA



fragment containing this BOX element using the primers 4144 and Eiv2 (Table S2). This



fragment was used as template in a new PCR reaction with the primers Box1 and Box2,



containing BamHI sites in their 5’-ends, resulting in specific amplification of the qsr



boxAB2C element. This fragment was ligated into pCR2.1-TOPO vector (Invitrogen)



giving rise to plasmid pCRAB2C. pCRAB2C derivatives containing deleted variants of



the AB2C motif were then generated using a PCR-restriction protocol as follows. To



remove any of the four boxes in the AB2C motif, primer pairs that annealed to DNA



regions flanking the box modules to be deleted were first designed. The oligonucleotide

primers, each complementary to opposite strands of the pCRAB2C plasmid, were used to



replicate both plasmid strands by PCR, thereby generating a plasmid with staggered



nicks. Since the primer pairs were designed to contain a unique restriction site at their 5’



ends, subsequent treatment of the PCR product with the appropriate restriction enzyme



efficiently removed the box module(s) lying between the 5’ ends of the two primers used



in the PCR reaction. Next, the PCR product was treated with DpnI to remove template



DNA, and purified by agarose gel electrophoresis. Finally, the plasmid was religated and



transformed into E. coli Top 10 competent cells (Invitrogen). This PCR-restriction



strategy was first applied to construct pCRAB2C derivatives containing AB2 (pCRAB2),



B2C (pCRB2C) and AC (pCRAC) box motifs, using the primer pairs Fjcf/Fjcr (contains a



StuI 5’ restriction site), Fjaf/Fjar (contains a NdeI 5’ restriction site) and Fjbf/Fjbr



(contains a StuI 5’ restriction site) respectively. To construct a derivative containing a



boxB2 motif (pCRB2), we used the pCRAB2 plasmid as a template in a PCR together with



the primer pair Fjaf/Fjar. The various box combinations were isolated from their



respective recombinant plasmid by digestion with BamHI, and ligated in either



orientation into the BamHI site downstream of the PE promoter in pOE4144 (for details



see Knutsen et al. (2)). A pOE4144 derivative containing a boxAB7C motif was



constructed by PCR amplification of a boxAB7C element located upstream of the spr1604



locus in the S. pneumoniae R6 genome. First, a 600 bp DNA fragment encompassing the



AB7C motif was amplified using the primers Box7.1 and Box7.2. This DNA fragment



was subsequently used as a template for specific amplification of the boxAB7C element



using primers (Box7.3 and Box7.4) containing BamHI sites in their 5’-ends. The



fragment was treated with BamHI, and ligated in either orientation into the BamHI site of

pOE4144. All the pOE4144 derivatives constructed in this work were integrated into the



genome of S. pneumoniae strain EK100 by homologous recombination in the region



upstream of the qrsAB promoter.







Construction of transcriptional fusions and modifications of boxABC at the comAB



locus



The OE4151 strain, which contains a promoterless lacZ gene inserted into the



pneumococcal genome behind a comAB promoter lacking boxABC, and the positive



control strain OE4150, which is identical to OE4151 except that boxABC is left intact,



were constructed as follows. A 1302 bp DNA fragment from the comAB locus including



the first fifty-eight 5’-nucleotides of comA together with the complete comAB promoter



and its upstream region was amplified from the CP1200 genome using the primers



ComA7 and ComA8. This fragment was restricted with NsiI and BamHI, and ligated into



the corresponding sites of the vector Litmus 28 (New England Biolabs), giving rise to the



recombinant plasmid pLicom1. To remove the boxABC element, pLicom1 was



subsequently used as a template in a PCR reaction with the primer pair ComA3/ComA4



(contains a NheI 5’ restriction site) using the same technique as described above. The



PCR products were digested with DpnI to remove template DNA, and NheI to remove the



ABC box motif. Agarose gel purified products were next religated, and transformed into



E. coli TOP10 cells, giving rise to pLicom2. The inserts in pLicom1 and pLicom2 were



isolated by digesting the plasmids with HindIII and BamHI, and purified by agarose gel



electrophoresis. Next, the fragments were ligated into the corresponding restriction sites



upstream of the promoterless lacZ gene in the nonreplicating pEVP3 vector, resulting in

the constructs pEVP3-4150 and pEVP3-4151, respectively. Finally, natural



transformation was used to integrate pEVP3-4150 and pEVP3-4151 into the chromosome



of the S. pneumoniae EK100 strain by homologous recombination, giving rise to the



mutant strains OE4150 and OE4151.



The OE4061 strain, which lacks the BOX-element upstream of comAB, and the



positive control strain OE4060, which is identical to OE4061 except that boxABC is left



intact, were derived from strain CP1200 as follows. A 1 kb DNA fragment containing the



complete comAB promoter and the 5’-half of the comA gene was amplified using the



primers comA1 and comA2. The fragment was digested with NsiI and ligated into



pLitmus 28 (New England Biolabs), resulting in the plasmid pLicom3. To construct a



pLicom3 derivative (pLicom4) harboring a comAB promoter region lacking boxABC,



pLitcom 3 was used as template in a PCR-deletion protocol identical to the one used for



generating pLitcom2. The inserts in pLicom3 and pLicom4 were next isolated by



digesting the plasmids with NsiI, purified by agarose gel electrophoresis, and ligated into



the corresponding restriction site in the vector pEVP3, resulting in the derivatives



pEVP3-4160 and pEVP3-4161, respectively. These plasmids were integrated into the



chromosome of S. pneumoniae CP1200 by natural transformation, giving rise to the



mutant strains OE4160 and OE4161. Upon integration of pEVP3-4160 and pEVP3-4161



into the CP1200 genome in the comA gene, the promoter regions originating from



pEVP3-4160 and pEVP3-4161 were inserted in front of fully functional comAB genes.



To monitor spontaneous competence development in the OE4160 and OE4161



strains, a competence inducible luciferase reporter gene was next integrated into the



chromosome of both mutants. A derivative of the pR424 recombinant plasmid (1, 6) was

constructed for this purpose (see Table S1). pR424 contains the Photinus pyralis luc gene



placed under control of the competence inducible promoter of the late com gene ssbB.



The chloramphenicol resistance gene in pR424 was exchanged with the spectinomycin



(spc) resistance gene from pR412 (3). First, the spc gene was amplified from pR412



using the primers Spec1 and Spec2. The PCR products were subsequently digested with



PstI and HindIII, and ligated into the corresponding sites of pR424. The resulting



plasmid, pR459, was then transformed into the OE4160, OE4161, and CP1200 strains.



Homology-dependent integration of pR459 into the ssbB locus resulted in strains



OE4170, OE4171, and OE4180, respectively (Table S1). All mutants constructed in this



work were verified by DNA sequencing.







Transformation of S. pneumoniae



An overnight culture of the pneumococcal strain to be transformed was diluted to an



OD550 of 0.05 in prewarmed (37°C) CAT broth. Before samples were withdrawn for



transformation, reconstitution of growth was allowed by incubating 1 ml samples at 37°C



for 30 min. Genomic or plasmid DNA was added to a final concentration of 2 to 5 µg ml–

1

together with 250 ng of CSP-1 ml–1. Cells were incubated for 2.5 h before plating on



CAT-agar plates containing the appropriate antibiotics for selection.







Reporter assays



β-galactosidase assays were carried out as described previously (2). Hydrolysis of ONPG



was recorded in a spectrophotometer at 420 nm, and enzyme activity was calculated



according to the method of Miller (4).

Strains used for luciferase assays were grown to OD550 = 0.4, aliquoted, and



stored as glycerol stocks at -80C. Prior to freezing, cells were washed 10 times in cold



CAT medium to remove any endogenously produced CSP from the culture supernatant.



Detection of luciferase activity was essentially performed as described previously (1, 6).



After thawing glycerol stocks, 100 l of stored cells were pipetted into Eppendorf tubes,



pelleted by centrifugation, and resuspended in 1 ml fresh CAT medium supplemented



with 0.2% (w/v) bovine serum albumin. For each test sample, 280 µl diluted culture was



mixed with 20 µl of firefly D-luciferin (10 mM solution in growth medium) and



transferred into a 96-well Corning NBS plate with clear bottom. The plate was incubated



at 37°C in an Anthos Lucy 1 luminometer for 7.5 hours. Optical density (OD492) and



luminescence were measured automatically by the luminometer at 10-minute intervals.





REFERENCES



1. Chastanet, A., M. Prudhomme, J.P. Claverys, and T. Msadek. 2001. Regulation of

Streptococcus pneumoniae clp genes and their role in competence development and stress

survival. J. Bacteriol. 183: 7295-7307.

2. Knutsen, E., O. Ween, and L.S. Håvarstein. 2004. Two separate quorum-sensing

systems upregulate transcription of the same ABC transporter in Streptococcus

pneumoniae. J. Bacteriol. 186: 3078-3085.

3. Martin, B., M. Prudhomme, G. Alloing, C. Granadel, and J.P. Claverys. 2000.

Cross-regulation of competence pheromone production and export in the early control of

transformation in Streptococcus pneumoniae. Mol. Microbiol. 38: 867-878.

4. Miller, J.H. 1972. Experiments in molecular genetics. Cold Spring Harbor Press, Cold

Spring Harbor, N.Y.

5. Morrison, D.A., S.A. Lacks, W.R. Guild, and J.M. Hageman. 1983. Isolation and

characterization of three new classes of transformation-deficient mutants of

Streptococcus pneumoniae that are defective in DNA transport and genetic

recombination. J. Bacteriol. 156:281-290.

6. Prudhomme, M. and J. P. Claverys. 2006. There will be a light: the use of luc

transcriptional fusions in living pneumococcal cells, p. in press. In R. Hakenbeck and G.

S. Chhatwal (ed.), The Molecular Biology of Streptococci. Horizon Scientific Press.

7. Sambrook, J., E.F. Fritsch, and T. Maniatis. 1989. Molecular cloning, vol. 3. Cold

Spring Harbor Laboratory Press, Cold Spring Harbor, N.Y.



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