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Aerosols

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Aerosols
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posted:
11/25/2011
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Dr. Fangqun Yu

Atmospheric Sciences Research Center



Sponsor: Department of Energy, Office of Biological and Environmental Research (BER)

Dates: August 15, 2009 – August 14, 2011

Amount: $318,858



Coupling an advanced particle microphysics model with WRF-Chem and im-

proving aerosol-climate interaction simulations at regional scales



Simulation of global and large-scale features of climate change has improved considerably

over the past decade; however, climate models do not yet accurately simulate important features

of regional climate variability and change. Anthropogenic aerosols can substantially reduce the

surface solar irradiance, alter the vertical solar heating profile and cloud properties, and modify

the hydrological cycle. The impact of aerosols on the Earth’s climate depends strongly on the

particle properties (size distribution, composition, and mixing state), and is a major source of un-

certainties in weather and climate predictions. In order to predict the current and future regional

climate with high degree of confidence, the key processes controlling spatial and temporal distri-

butions of tropospheric particles and aerosol–climate interactions have to be properly represented

in regional climate models. The release of Weather Research and Forecasting (WRF)-Chem

Model opens new possibilities for studying the interactions of meteorology, aerosol, cloud, radia-

tion, and chemistry in a fully interactive manner over a wide range of spatial and temporal scales.

Under this project, we propose to improve simulations of the aerosol processes in the WRF-

Chem and to investigate the aerosol-climate interactions at regional scales. We will first incorpo-

rate a computationally efficient advanced particle microphysics (APM) model into the frame-

work of the WRF-Chem as an additional aerosol scheme. The APM model, which has been re-

cently incorporated into a global chemistry model (GEOS-Chem), is a sectional model designed

for studying relative contributions of secondary and primary particles to the abundance of cli-

mate effective aerosols. The model contains state-of-the-art nucleation modules and simulates

the coating of primary particles by volatile species. Using the WRF-Chem with new aerosol

scheme, we will then simulate the evolution of size-resolved secondary and primary particle

properties in the atmosphere over the United States. The model results will be assessed and vali-

dated with the relevant measurements obtained in several field campaigns. Finally we will study

the aerosol-climate interactions at regional scales, using existing modules in WRF-Chem that

link aerosol sizes and chemical composition predicted by the APM model to the aerosol optical

properties, radiative transfer, cloud optical properties, and precipitation.

The proposed research will result in the improved representation of aerosol processes and

hence aerosol-climate interactions in the community regional climate model WRF-Chem and a

substantial reduction of the uncertainties in the assessment of the climatic impact of anthropo-

genic emissions. This project is directly relevant to the BER long term measure "to deliver im-

proved scientific data and models about the potential response of the Earth's climate and terre-

strial biosphere to increased greenhouse gas levels for policy makers to determine safe levels of

greenhouse gases in the atmosphere."









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