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VNCI Responsible Care Award 2010



SECTION 0 - Submission details



Akzo Nobel Industrial Chemicals B.V., Amersfoort

Submission title New generation anti caking agent for salt

Main contact details Name: Frank Hoks Location: Amersfoort

for administration Director Technology Salt

Tel: +31334676966 e-mail frank.hoks@akzonobel.com

Address: P.O. Box 247; Stationsstraat 77, 3800 AE Amersfoort









SECTION 1 – Brief introduction AkzoNobel Industrial Chemicals



AkzoNobel Industrial Chemicals produces salt and energy, chlor-alkali products and derivatives like

monochloroacetic acid (MCA). It is Europe’s largest producer of vacuum salt and a leading supplier of

chlorine, caustic lye, hydrochloric acid, ferric chloride and water treatment chemicals and MCA used in

the chemical, detergent, construction, food, pulp and paper and plastic industries. Its products are

essential in daily life and used in the manufacture of among others vehicles, glass, performance

plastics, pharmaceuticals, textiles and in disinfectants for swimming pools.

Employing approximately 1,800 people, Industrial Chemicals has production sites at Rotterdam,

Hengelo and Delfzijl in the Netherlands, Ibbenbüren, Frankfurt and Bitterfeld in Germany, Mariager in

Denmark, LeMoyne in the USA, and Taixing in China.





SECTION 2 – Description of improvement



The Challenge

Salt, being a very pure product, has a natural tendency to cake when it is put in stock. Caking, the

process where salt-crystals are sticking together, is an undesired process as it causes hard lumps of

salt and it hampers the handling of salt in terms of storage, loading, transport and discharging from

ships or trucks.



In order to prevent caking of salt a so called anti caking agent is added. Only very small amounts are

needed. Usually 3 to 5 parts per million (ppm) are sufficient to keep the salt free flowing, which is

crucial to keep the logistic part of the salt business in motion.



It was KNZ, one of our AkzoNobel forefathers, who in 1957 invented and patented ferro cyanide

Fe(CN)6 as a very powerful and effective anti caking agent, still today’s world wide standard.



With today’s applications and technologies however ferro cyanide has certain draw backs which made

AkzoNobel Industrial Chemicals to invest in an extensive R&D program in order to try to find an even

better successor.

Our salt is used in state of the art membrane electrolysis processes for the production of chlorine and

caustic lye. When the stable ferro cyanide complex enters the membrane cells the circumstances are

so harsh that it is broken down in parts. The free iron has distinct negative effects since it is deposited

on or in the membranes which increases the power consumption.



Delta cell voltage between electrolyzer with and without Fe(CN)64-

at 6 kA/m2

120



Start test



Delta cell voltage

100

Stop test



Out of operation

80

Delta cell voltage (mV)









60









40









20









0

24-3-2006 13-5-2006 2-7-2006 21-8-2006 10-10-2006 29-11-2006 18-1-2007 9-3-2007 28-4-2007 17-6-2007 6-8-2007









The picture shows a clear increase in cell voltage/ power consumption due to deposit of iron under

th

test-conditions. (ref.: Meijer, J.A.M., Next generation anti-caking: Meso Tartrate, 9 International

Symposium on Salt, Beijing, September 2009, ISBN 978-7-80251-213-9)



The cyanide is transformed into harmful nitrogentrichloride that may lead to explosions under certain

conditions, as incidents, happened in the nineties (explosion of a rail tanker in Belgium, explosion of a

vaporizer in Germany) demonstrate. (ref. Piersma, H., Nitrogen Trichloride: a Continuing Challenge,

Eurochlor Fifth technical seminar, Barcelona, 8-9 February 2001.



In another field of application of the salt, high way de-icing, where the salt reverts into the

environment, the call for biodegradability is getting louder and louder.



All excellent reasons for us, as the undisputed leader of vacuum salt for the Chemical Transformation

market and important supplier in the road salt market, to take up the challenge of developing a new

generation anti caking agent for salt!









2

The improvement:

The last couple of years AkzoNobel Industrial Chemicals developed and patented a new, advanced

anti caking agent: Fe-mTA (Ferro-meso-Tartrate), in short mTA. It is a complex of iron and meso-

tartrate, working according to the same principles as the classic Ferro cyanide does: The iron (Fe) is

protected and carried by, in this case, the tartrate complex to the salt crystals where the iron can

perform its anti-caking effect by “disturbing” the crystal-grid of the salt, thus caking is prevented.



The main difference with the classic ferro cyanide is in the stability of the complex. Ferro cyanide is a

very stable molecule and hard to break down, which makes it difficult to prevent it from entering into

the membrane cells of electrolysis plants. Also in nature, though in very low concentrations, it is hardly

degradable.



The mTA however, decomposes easily whenever the salt is dissolved to brine, the iron can easily be

filtered out, the organic tartrates degrade and evaporate harmlessly.



All in all, the new product is totally free of cyanides, the iron can be prevented from entering the

sensitive membrane electrolysis processes and in nature, on the roads, the product will vanish by

simple biological degradation.





The team

As referred to above, the first initiatives and try-outs were carried out on lab scale at our Deventer

based Salt R&D department. A first scaling-up has been performed by starting delivery of the so called

mTA-salt from our Delfzijl salt producing facility to the membrane electrolysis plants of AkzoNobel

Industrial Chemicals in Rotterdam, The Netherlands.



A recent breakthrough in the recipe led to a further improvement of the anti-caking functionality of the

product, enabling further external roll-out.



The project can be characterized as being a real multi disciplinary project. R&D, production and

technology, marketing and sales, purchasing, IP are all highly engaged as from the early start of the

project, expressing the high degree of integration of this project throughout the whole salt – chlorine

production chain.





The benefits

In brief the following benefits are in focus:

 Safety: Intrinsic safety improvement at electrolysis processes in general due to the absence of

cyanides, eliminating one source of nitrogen able to convert to nitrogentrichlorides, leading to

a potential explosion risk.

 Energy: Substantial lower power consumption at membrane electrolysis processes. Potential

annual electricity saving for the European chlorine industry amounts up to ca. 350 – 500 GWh,

corresponding to 160 – 230 kton CO2e reduction, or in financial terms a saving of approx. 17

– 25 Mio. Euro (based on 50 Euro/MWh).

 Profit: Next to the obvious saving on energy costs: The increased lifetime of membranes and

electrodes, reducing waste and downtime.

 Environment: Environmental friendly and bio-degradable alternative for highway de-icing

applications.









3

Fit to AkzoNobel’s values

The mTA project has an excellent fit with our company values. Initiated by the courage to question,

drafting the challenge, our salt-customers in primary focus, addressing their sustainability-needs of

tomorrow. Finding an innovative solution and rolling out the implementation in an entrepreneurial way.

And while doing so, in an honest and responsible manner, we continuously develop the talents of our

people in this exciting project.





Implementation details

Longer term operational and stable experiences in the electrolysis process of AkzoNobel in Rotterdam

were very positive as Fe-deposits in the membrane cells indeed could be avoided, with the result of a

considerable saving of electrical energy, as mentioned before.





Initially the anti-caking behavior of the salt was not yet as good as with the classic ferro cyanide,

resulting in some more hassle during unloading of vessels.

Transport tests with a so called self unloading vessel showed clearly the room for improvement:









A continuous effort was made in our R&D department since then, in order to find an optimized recipe.

In the summer of 2008 a breakthrough was realized in producing this improved product .



Recently performed similar transport tests show far better results:









This substantial improved anti-caking performance now enables a further roll out towards more

customers and applications down the chain, as mentioned before.









4

Recognition by the chemical industry



While further testing takes place, like storage tests, test deliveries to potential customers, filtration- and

de-icing tests, market introduction is carefully prepared.



th

A very successful step in this process was our presentation and launch of mTA at the 9 International

Symposium on Salt in Beijing, China, September 2009. To a broad audience of salt and chemical

producers we presented our experiences at a scientific presentation, held a press conference and

elucidated on the advantages in different applications. A lot of attention and interest was expressed by

the market.

(ref. annex 1)









A lot of interest at our booth in Beijing





In January 2010 we launched mTA in the US high way de-icing market, by a scientific presentation at

the annual meeting of the US Transport Research Board, Washington DC. The first responses from

these decision makers in winter road maintenance were positive.

(ref. annex 2)



Next to the own AkzoNobel deliveries in March 2010 the first sizeable contract with another major

European chlorine producer became reality for the delivery of half a million ton mTA salt/year. As a

consequence already in 2010 1.5 million tons of mTA salt will find its way to membrane electrolyses in

Europe.





In summary

To summarize, it can be stated that after a period of hard work and first positive experiences, an

innovative breakthrough in the performance of the product brought the project in a new phase.

A phase of materializing and implementing a sustainability driven R&D concept into real business.

Business in the highly integrated salt-chlorine chain and in highway de-icing, product stewardship “pur

sang”.



Technology pushing, in balance with a market pulling, a challenging but very exciting example of

making “Tomorrow’s Answers Today” work in AkzoNobel’s field of sustainability and responsible care.







5

SECTION 3 – Contribution to AkzoNobel’s ambitions in the field of sustainability and

responsible care.

The development of the mTA-Salt supports the following sustainability and responsible care ambitions

of AkzoNobel Industrial Chemicals:



Sustainability and Responsible Care Ambitions

1 Zero approach in HSE: by eliminating Ferro cyanide mTA-salt contributes to a safe working

environment at the plants of our customers, by intrinsically minimizing the risk of explosion

due to NCl3.

2 Reduce Greenhouse Gas emissions: The usage of mTA-Salt instead of salt with Ferro

Cyanide results in lower energy consumption at the plants of our customers without having

other drawbacks. CO2 foot print of the European chlorine sector potentially improves with a

reduction of 160 - 230 kton CO2 per year.

3 Low environmental footprint: because mTA-salt is biodegradable, when applied to de-icing

salt on highways the ecological footprint of this salt is improved substantially when compared

to de-icing salt with Ferro cyanide.

4 BU Industrial Chemicals wants to be a leader in the field of sustainable solutions, and it has

clearly demonstrated this ambition with the development of mTA-salt. In the demanding

sector as the chlorine industry is, where safety is of utmost importance, it is not easy to

implement a new product. The fact that mTA-salt succeeded is a big breakthrough and this

new product will raise the bar in the industry.









Annex 1: Media Coverage ISS 2009

Annex 2: Brochure “The green alternative for anti-caking in road salt”









6



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